Well if we're talking about songs; my vote goes to Sakuran. I think it'd be right at home in the Mayonaka single, which it seems many agree is the best single in Ringo's career.
HF Gamble, Hatsukoi Shoujo, and Karisome Otome deserve mention too; if those 4 songs would have been a separate release, I would have considered it top tier.
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